Nature Communications - Stabilizing silicon without sacrificing other device parameters is essential for practical use in lithium and post lithium battery anodes. Here, the
This work describes a new strategy to achieve both safe and energy-dense battery (SEB) cells, as schematically sketched in Fig. 1, where the cell resistance is plotted against the inverse of temperature rst, a passivated cell is judiciously designed and built by using highly stable materials and by creating exceptionally stable EEIs, as characterized by
Introduction. With the highest specific capacity (3860 mAh g −1) and the lowest redox potential (−3.04 V versus the standard hydrogen potential), lithium (Li) metal anode is considered as the ultimate choice for high-energy batteries. 1-4 However, its application is hindered by the Li dendrite growth during cycling, which stems from unavoidable Li/electrolyte
High performance flexible lithium-ion battery electrodes: ion exchange assisted fabrication of carbon coated nickel oxide nanosheet arrays on carbon cloth. Adv. Funct. Mater., 31 (24) (2021), p. 2101199, 10.1002/adfm.202101199. View in Scopus Google Scholar [38]
It is worth noting that the lithium–oxygen battery reported here can operate under capacity levels as high as 5,000 mAh g carbon −1 with an average discharge voltage of 2.7 V, leading to a
The increasing demand for large-capacity lithium batteries requires new anode materials satisfying both high capacity and long-life cycles. Here, a free-standing, binder-free, and environmentally friendly carbonized eggshell membrane (CEM) anode with a highly conductive interwoven network is presented for the use in high-performance lithium batteries.
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We prepared the polyacrylonitrile (PAN)/cellulose composite separator for lithium-ion batteries (LIBs) using electrospinning and examined its thermal stability, ionic conductivity, electrochemical stability and battery performance, toward high performance of the LIB. The thermal stability of the separator was enhanced by introducing the cellulose at the
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Rechargeable batteries are widely regarded as an electrochemical energy storage method to mitigate fossil fuel pollution [1].However, lithium-ion batteries (LIBs) have nearly reached their energy density limit (theoretically ≈ 390 Wh kg –1) [2], making it challenging to meet the increasing demand for higher energy density in portable electronic devices and
Beyond lithium-ion technologies, lithium–sulfur batteries stand out because of their multielectron redox reactions and high theoretical specific energy (2500 Wh kg–1). However, the intrinsic irreversible transformation of soluble lithium polysulfides to solid short-chain sulfur species (Li2S2 and Li2S) and the associated large volume change of electrode materials
Developing high-performance lithium-ion batteries (LIBs) with high energy density, rate capability and long cycle life are essential for the ever-growing practical application. Among all battery components, the binder plays a key role in determining the preparation of electrodes and the improvement of battery performance, in spite of a low usage amount. The
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Lithium-ion batteries have been extensively employed for past two decades [1], [2], while the charge-storage mechanism of (de-)intercalation mode limits its capacity property.With high theoretical gravimetric energy density of 2600 Wh kg −1 and high theoretical capacity of 1672 mAh g −1, meanwhile the application of abundant and low-cost sulfur as
The pursuit of high energy density has promoted the development of high-performance lithium metal batteries. However, it faces a serious security problem. The resulting lithium-O 2 battery achieved a high coulombic efficiency of 99.5% and a significantly increased capacity retention from 45% to 60% over 100 cycles [101].
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Electrolyte engineering improved cycling of Li metal batteries and anode-free cells at low current densities; however, high-rate capability and tuning of ionic conduction in
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Lithium (Li) metal battery is highly pursued as the next-generation power source 1,2.However, the implementation of Li metal anode is hindered by poor cycle life, which originates from
High-capacity lithium-containing alloy anodes (e.g., Li4.4Si, Li4.4Sn, and Li3P) enable lithium-free cathodes (e.g., Sulfur, V2O5, and FeF3) to produce next-generation lithium-ion batteries (LIBs) with high energy density. Herein, we design a Li3P/C nanocomposite with Li3P ultrafine nanodomains embedded in micrometer-scale porous carbon particles. Benefiting from
The commercial development of lithium-sulfur batteries (Li-S) is severely limited by the shuttle effect of lithium polysulfides (LPSs) and the non-conductivity of sulfur. Herein, porous g-C3N4 nanotubes (PCNNTs) are synthesized via a self-template method and utilized as an efficient sulfur host material. The one-dimensional PCNNTs have a high specific surface area (143.47
Lithium–ion battery (LIB) is regarded as the most promising candidate of the clean, green, and renewable energy, which is attributed to its high specific capacity, long life cycle, low temperature discharge performance, and excellent capacity retention [3,4,5,6]. Currently, graphite is generally used as the anode material for commercialized
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These channels can serve as facile and selective Li-ion diffusion pathways on the surfaces of lithium anodes, thereby ensuring stable lithium stripping/plating even at high areal current densities. CMP-modified lithium anodes (CMP-Li) exhibit cycle stability of 2550 h at an areal current density of 20 mA cm −2. Furthermore, CMP is readily
Lithium-oxygen (Li-O2) batteries have been regarded as an expectant successor for next-generation energy storage systems owing to their ultra-high theoretical energy density. However, the comprehensive properties of the commonly utilized organic salt electrolyte are still unsatisfactory, not to mention their expensive prices, which seriously hinders the
Development of high-performance lithium metal batteries with a wide operating temperature range is highly challenging, especially in carbonate electrolyte. Solid polymer electrolyte with in-situ generated fast Li+ conducting network enable high voltage and dendrite-free lithium metal battery. Energy Storage Materials 2022, 44, 93-103
Lithium–sulfur batteries with high theoretical energy density are attracting more and more attention as candidate materials for next-generation energy storage systems. However, the insulating properties and poor shuttle effect of sulfur are still the main challenges faced by high-performance lithium–sulfur batteries. For this reason, we developed 3D MXene/T-CNF
For simplicity a fixed ratio of lithium ions (Li +) to ethylene oxide (EO) of 0.10 was maintained in the materials by addition of the lithium salt, Lithium Nitrate (LiNO3), which is widely
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